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• W4307773293 abstract "Developing low-cost all-iron hybrid redox flow batteries (RFBs) presents a practical alternative to the high-cost all-vanadium RFBs and is deemed vital for grid-scale energy storage applications. However, the intrinsically poor Fe anode reversibility associated with the deposition and dissolution of metallic iron greatly limits the cycling performance and long-term stability of all-iron hybrid RFBs. Herein, a highly reversible and dendrite-free Fe anode is reported for all-iron RFBs through regulation of polar solvent dimethyl sulfoxide (DMSO) on FeCl2 anolyte, which simultaneously reshapes Fe2+ solvation structure and induces controllable oriented Fe deposition. Combining both experimental and theoretical analyses, the polar DMSO additives prove effective in replacing H2 O molecule from the primary solvation shell of Fe2+ cation via the Fe2+ -O (DMSO) bond and meanwhile induces a fine-grained Fe nucleation on the preferred Fe (110) plane, which are responsible for the minimized hydrogen evolution and dendrite-free Fe deposition that significantly enhance Fe anode reversibility. The all-iron RFB based on the proposed FeCl2 -DMSO anolyte demonstrates an excellent combination of peak power density of 134 mW cm-2 , high energy efficiency of 75% at 30 mA cm-2 , and high capacity retention of 98.6% over 200 cycles, which presents the best performance of all-iron RFBs among previously reported research." @default.
• W4307773293 created "2022-11-05" @default.
• W4307773293 creator A5028571695 @default.
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• W4307773293 date "2022-10-30" @default.
• W4307773293 modified "2023-10-17" @default.
• W4307773293 title "Simultaneous Regulation of Solvation Shell and Oriented Deposition toward a Highly Reversible Fe Anode for All‐Iron Flow Batteries" @default.
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• W4307773293 doi "https://doi.org/10.1002/smll.202204356" @default.
• W4307773293 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36310140" @default.
• W4307773293 hasPublicationYear "2022" @default.
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