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• W4307840946 abstract "Carbon-coated metal chalcogenide composites have been demonstrated as one type of promising anode material for sodium-ion batteries (SIBs). However, combining carbon materials with micronanoparticles of metal chalcogenide always involve complicated processes, such as polymer coating, carbonization, and sulfidation/selenization. To address this issue, herein, we reported a series of carbon-coated FexSey@CN (FexSey = FeSe2, Fe3Se4, Fe7Se8) composites prepared via the thermodynamic transformation of a crystalline organic hybrid iron selenide [Fe(phen)2](Se4) (phen = 1,10-phenanthroline). By pyrolyzing the bulk crystals of [Fe(phen)2](Se4) at different temperatures, FexSey microrods were formed in situ, where the nitrogen-doped carbon layers were coated on the surface of the microrods. Moreover, all the as-prepared FexSey@CN composites exhibited excellent sodium-ion storage capabilities as anode materials in SIBs. This work proves that crystalline organic hybrid metal chalcogenides can be used as a novel material system for the in situ formation of carbon-coated metal chalcogenide composites, which could have great potential in the application of electrochemical energy storage." @default.
• W4307840946 created "2022-11-06" @default.
• W4307840946 creator A5001558626 @default.
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• W4307840946 date "2022-11-01" @default.
• W4307840946 modified "2023-10-18" @default.
• W4307840946 title "Thermodynamic Transformation of Crystalline Organic Hybrid Iron Selenide to Fe_<i>x</i>Se_<i>y</i>@CN Microrods for Sodium Ion Storage" @default.
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• W4307840946 doi "https://doi.org/10.1021/acsami.2c15688" @default.
• W4307840946 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36317753" @default.
• W4307840946 hasPublicationYear "2022" @default.
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