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- W4308040919 endingPage "155491" @default.
- W4308040919 startingPage "155491" @default.
- W4308040919 abstract "Silicon-based (Si-based) materials have aroused extensive attention owing to their ultra-high theoretical specific capacity, while the huge volume expansion and inferior electronic conductivity have impeded their practical application in lithium-ion batteries (LIBs). Rational structural design has been regarded as a fascinating strategy, especially for yolk-shell structures. Herein, Si nanoparticles (Si NPs) were encapsulated in ZIF-67 metal–organic frameworks to obtain [email protected] particles, which were wrapped in one-dimensional carbon fibers (CFs) by simple processes of electrospinning, vulcanization and carbonization to obtain a free-standing [email protected]9S8 CF electrode. The yolk-shelled [email protected]9S8 particles could remarkably ameliorate the volume variation of Si materials during the lithiation/de-lithiation cycling and the introduction of CFs endowed an efficient one-dimensional electronic pathway accurately to improve the conductivity of composite materials. In addition, it was not negligible that the as-obtained [email protected]9S8 CF films could be as a self-supporting electrode, which avoided the traditional cumbersome procedure of the electrode preparation. The resulting composite electrodes possess an excellent rate performance and an ultra-stable cycling lifespan. We hope this work can provide some novel insights for the development of the self-supporting Si-based electrode materials." @default.
- W4308040919 created "2022-11-07" @default.
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- W4308040919 date "2023-02-01" @default.
- W4308040919 modified "2023-10-16" @default.
- W4308040919 title "Encapsulating yolk-shelled Si@Co9S8 particles in carbon fibers to construct a free-standing anode for lithium-ion batteries" @default.
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- W4308040919 doi "https://doi.org/10.1016/j.apsusc.2022.155491" @default.
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