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- W4308155995 abstract "Highly efficient removal of mercury ion (Hg2+) from aqueous solution is a serious concern. Herein, a novel metal-organic framework (MOF) containing dual sulfur sites was successfully constructed via an in-situ method. Different with previous reports, thiophene and thiol sites were simultaneously introduced via organic linker and inorganic cluster, resulting in high-density sulfur sites. The composition and porosity of the newly synthesized DUT-67-SH (DUT, Dresden University of Technology) were systematically characterized. Based on abundant sulfur sites and strong host-guest interaction, DUT-67-SH exhibits a high adsorption capacity (370.2 mg g-1) and rapid adsorption kinetics (∼3 min for equilibrium). Excellent separation selectivity, regenerability, and applicability under wide acidic pH range were further confirmed. Mechanism analysis suggests that the chemical bonding between sulfurs and Hg2+ is the main driven force. Thus, our work demonstrates that DUT-67-SH is a potential adsorbent for Hg2+, and more importantly, provides a new insight for introducing high-density sulfur sites in MOFs." @default.
- W4308155995 created "2022-11-08" @default.
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- W4308155995 date "2023-02-01" @default.
- W4308155995 modified "2023-10-18" @default.
- W4308155995 title "Construction of dual sulfur sites in metal–organic framework for enhanced mercury(II) removal" @default.
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- W4308155995 doi "https://doi.org/10.1016/j.jcis.2022.10.153" @default.
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