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- W4308298768 abstract "<p indent=0mm>The C<sub>19</sub>-diterpenoid alkaloids belong to a class of natural products with significant biological activities. These molecules are structurally characterized by complex cage-like skeletons and dense functional substituents. The efficient preparation of the A/E aza-bridged ring system, which is ubiquitous in C<sub>19</sub>-diterpenoid alkaloids, would lay an important foundation for their total synthesis. This paper reports a new asymmetric synthesis of the functionalized A/E bicyclic fragment of the C<sub>19</sub>-diterpenoid alkaloids, featuring desymmetrization, diastereoselective allylaltion, aldol hydroxymethylation, and reductive amination as key steps." @default.
- W4308298768 created "2022-11-10" @default.
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- W4308298768 date "2023-02-24" @default.
- W4308298768 modified "2023-09-27" @default.
- W4308298768 title "Asymmetric synthesis of the functionalized A/E bicyclic fragment of the C<sub>19</sub>-diterpenoid alkaloids" @default.
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- W4308298768 doi "https://doi.org/10.1360/ssc-2022-0199" @default.
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