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• W4308305946 endingPage "119325" @default.
• W4308305946 startingPage "119325" @default.
• W4308305946 abstract "Phosphorus (P) harvesting from source-separated urine to optimize the overall nutrient loop is one of the most appealing benefits and is a global research interest in wastewater management and treatment. However, current P precipitation is mainly oriented to struvite, which is limited by the issues such as relatively low product purity and high cost of Mg source. Distinguished from previous conventional struvite precipitation, the strategy of precisely harvesting P from fresh human urine as high-purity calcium phosphate was first proposed in this study. This enhanced strategy can optimize P harvesting performance and product purity by simply regulating the consumption of calcium-based materials via model simulation and experimental validation. The thermodynamic model was constructed to probe the precipitation conversion mechanism, and visually predict the component and yield for products under various operating conditions. Batch experiments were conducted to investigate P recovery performance as a function of initial Mg2+ concentration, initial pH level, as well as degree of urine hydrolysis. Moreover, the alternative dosing scheme with different calcium salts and alkali was presented, diversifying the options for efficient P recovery. The results showed that, from the perspective of acidic storage for fresh urine, P recovery can be boosted along with eliminating urine hydrolysis. In urine with an initial pH=2.0, P can be completely recovered and purity for calcium phosphate can be optimized to 100% within a Ca/P ratio range of 1.67-2.3. Overall, this work is of great significance for precisely and efficiently harvesting P from urine and provides an integrated strategy for P resource recovery from urine." @default.
• W4308305946 created "2022-11-10" @default.
• W4308305946 creator A5045473616 @default.
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• W4308305946 date "2022-12-01" @default.
• W4308305946 modified "2023-09-23" @default.
• W4308305946 title "Phosphorus harvesting from fresh human urine: A strategy of precisely recovering high-purity calcium phosphate and insights into the precipitation conversion mechanism" @default.
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• W4308305946 doi "https://doi.org/10.1016/j.watres.2022.119325" @default.
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