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- W4308343604 abstract "Metal-support interaction has a substantial influence on catalyst activity while little attention has been paid to it in the plasma catalytic system. Herein, the effect of support on the activity of CoMnOX-based catalysts was investigated for trichloroethylene removal by plasma catalysis, and CoMnOX/ZSM-5 exhibited the highest mineralization rate (36.93−94.24 %), HCl and Cl2 yield (19.66−94.37 %), energy yield (63.29–29 g/kWh), as well as the lowest export ozone concentration (18.72–108.83 mg/m3) under 6–10 kV. The excellent catalytic activity of CoMnOX/ZSM-5 was ascribed to the formation of abundant defects and oxygen vacancies, which was induced by the SiOCo/Mn hybridization promoting Co/MnO bonds cleavage. CoMnOX/ZSM-5 also exhibited superior adsorption ability, large amount of Co3+, Mn4+ and adsorbed oxygen species, high reducibility and suitable acidity. Moreover, CoMnOX/ZSM-5 maintained superior water-resistant ability and high catalytic activity after 50 h operation. The proposed TCE degradation mechanism suggested that the contribution of plasma active oxygen species was involved in TCE oxidation and oxygen cycle of catalyst. This work provides a novel strategy to design catalysts in plasma catalytic system." @default.
- W4308343604 created "2022-11-11" @default.
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- W4308343604 date "2023-01-01" @default.
- W4308343604 modified "2023-10-02" @default.
- W4308343604 title "Enhanced activity of plasma catalysis for trichloroethylene decomposition via metal-support interaction of Si O Co/Mn bonds over CoMnOX/ZSM-5" @default.
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- W4308343604 doi "https://doi.org/10.1016/j.seppur.2022.122553" @default.
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