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- W4308344575 endingPage "126955" @default.
- W4308344575 startingPage "126955" @default.
- W4308344575 abstract "Nanoparticle-based superlattices have attracted extensive research efforts due to their versatile composition and packing-dependent optical, magnetic, electronic, catalytic, mechanical properties. Yet the experimental understanding of the thermodynamics and pathways of the crystallization processes for these systems, which govern their ultimate morphology, size, and packing structure, has for long remained underexplored. This minireview highlights recent integration of liquid-phase transmission electron microscopy, which allows for real-space, real-time direct imaging of the crystallization processes at the single-particle level, with simulation and the conceptual framework established by pioneers such as Dr. A. A. Chernov. Different aspects of superlattice formation were revealed by direct imaging for the first time, such as the existence of prenucleation precursor in nonclassical crystallization, surface energy-dependent growth, and coalescence, allowing for the charting of phase coordinates and thermodynamic quantities at the nanoscale. We discuss the similarities and differences of crystal growth behaviors in atomic and nanoparticle systems, as well as engineering opportunities to fashion, shape, and achieve quality control in superlattice formation from nanoparticles, for next-generation optical and mechanical metamaterials." @default.
- W4308344575 created "2022-11-11" @default.
- W4308344575 creator A5012971955 @default.
- W4308344575 creator A5022256556 @default.
- W4308344575 creator A5068290128 @default.
- W4308344575 date "2023-01-01" @default.
- W4308344575 modified "2023-09-24" @default.
- W4308344575 title "In-situ imaging of nucleation and growth of superlattices from nanoscale colloidal nanoparticles" @default.
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