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• W4308372883 abstract "Polyoxopalladates (POPs) are a class of self-assembling palladium-oxide clusters that span a variety of sizes, shapes and compositions. The largest of this family, {Pd84 }Ac , is constructed from 14 building units of {Pd6 } and lined on the inner and outer torus by 28 acetate ligands. Due to its high water solubility, large hydrophobic cavity and distinct 1 H NMR fingerprint {Pd84 }Ac is an ideal molecule for exploring supramolecular behaviour with small organic molecules in aqueous media. Molecular visualisation studies highlighted potential binding sites between {Pd84 }Ac and these species. Nuclear Magnetic Resonance (NMR) techniques, including 1 H NMR, 1 H Diffusion Ordered Spectroscopy (DOSY) and Nuclear Overhauser Spectroscopy (NOESY), were employed to study the supramolecular chemistry of this system. Here, we provide conclusive evidence that {Pd84 }Ac forms a 1 : 7 host-guest complex with benzyl viologen (BV2+ ) in aqueous solution." @default.
• W4308372883 created "2022-11-11" @default.
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• W4308372883 date "2022-11-30" @default.
• W4308372883 modified "2023-09-25" @default.
• W4308372883 title "Water‐soluble Self‐assembled {Pd₈₄}^Ac Polyoxopalladate Nano‐wheel as a Supramolecular Host" @default.
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• W4308372883 doi "https://doi.org/10.1002/anie.202214203" @default.
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• W4308372883 hasPublicationYear "2022" @default.
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