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• W4308387630 endingPage "2211387" @default.
• W4308387630 startingPage "2211387" @default.
• W4308387630 abstract "Solid-state batteries (SSBs) are regarded as next generation advanced energy storage technology to provide higher safety and energy density. However, a practical application is plagued by large interfacial resistance, owing to solid-solid interface contact between ceramics electrolytes and Li anode. Introducing polymer-based coating between electrolytes and Li anode is a feasible strategy to solve this issue. Unfortunately, current polymer is hard to achieve intimate contact at the atomic scale and lacks of a bridge to transfer Li+ quickly between electrolytes and polymer coating. This gives rise to sluggish Li+ transfer dynamics, huge interface impedance and greatly limits the effectiveness of this strategy. Herein, Poly(lithium 4-styrenesulfonate)(PLSS) is introduced between Li6.5La3Zr1.5Ta0.5O12 (LLZTO) electrolyte and Li anode. The theories and experiments prove the existence of strong coordinating interaction between SO3Li in PLSS and atoms on LLZTO surface. This interaction structures a bridge to migrate Li+ fast across LLZTO/PLSS interface and hence interface impedance is as low as 9 Ω cm2. Moreover, the electron-blocking feature of PLSS can prevent electrons from tunneling the LLZTO/PLSS interface and combining with Li+ to form dendrite within LLZTO. PLSS-base cells show improved long-life cycling for 4700 h at 0.1 mA cm−2 at room temperature." @default.
• W4308387630 created "2022-11-11" @default.
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• W4308387630 date "2022-11-07" @default.
• W4308387630 modified "2023-10-16" @default.
• W4308387630 title "A Bridge between Ceramics Electrolyte and Interface Layer to Fast Li ⁺ Transfer for Low Interface Impedance Solid‐State Batteries" @default.
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• W4308387630 doi "https://doi.org/10.1002/adfm.202211387" @default.
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