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- W4308453662 abstract "Abstract In this paper, we report a unique type of core-shell crystalline material that combines an inorganic zeolitic cage structure with a macrocyclic host arrangement and that can remove trace levels of iodine from water effectively. These unique assemblies are made up of an inorganic Archimedean truncatedhexahedron ( tcu ) polyhedron in the kernel which possesses six calixarene-like shell cavities. The cages have good adaptability to guests and can be assembled into a series of supramolecular structures in the crystalline state with different lattice pore shapes. Due to the unique core-shell porous structures, the compounds are not only stable in organic solvents but also in water. The characteristics of the cages enable rapid iodine capture from low concentration aqueous I 2 /KI solutions (down to 4 ppm concentration). We have studied the detailed process and mechanism of iodine capture and aggregation at the molecular level. The facile synthesis, considerable adsorption capacity, recyclability, and β- and γ-radiation resistance of the cages should make these materials suitable for the extraction of iodine from aqueous effluent streams (most obviously, radioactive iodide produced by atomic power generation)." @default.
- W4308453662 created "2022-11-12" @default.
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- W4308453662 date "2022-11-04" @default.
- W4308453662 modified "2023-10-09" @default.
- W4308453662 title "Water-stable porous Al24 Archimedean solids for removal of trace iodine" @default.
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- W4308453662 doi "https://doi.org/10.1038/s41467-022-34296-4" @default.
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