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• W4308463649 endingPage "155604" @default.
• W4308463649 startingPage "155604" @default.
• W4308463649 abstract "Ag@AgCl@g-C 3 N 4 composite was successfully fabricated and applied for recyclable detection-removal of organic pollutions via SERS sensing. The constructed structure provides more SERS-active sites for efficient SERS sensing performance, as well as enhanced plasmon-induced hot carrier separation efficiency for superior photocatalytic property. The composite shows promising potentials in cycling detection-removal of organic pollutants. • Ag@AgCl@g-C 3 N 4 composite is reported for the first time in recyclable detection-removal of organic pollutions via SERS sensing. • The constructed structure provides more SERS-active sites for SERS sensing. • The constructed structure contributes to hot carrier separation efficiency. The global environment is continuously being exposed to toxic organic pollutants, which also greatly threaten human health. Therefore, it is important to develop substrates for detection, identification, and removal of these organic pollutants. In this study, a multifunctional and reusable composite is prepared by anchoring Ag nanoparticles onto Cl-rich g-C 3 N 4 nanosheets (Ag@AgCl@g-C 3 N 4 ). The composites present not only excellent surface-enhanced Raman scattering (SERS) performance attributed to enhanced local electric field and SERS-active sites from the constructed structure, but also superior photocatalytic property boosted by the enhanced charge separation efficiency. These exceptional activities allow the composite to be used for detection of methylene blue with a high enhancement factor of 1.39×10 6 , and a limit of detection of 1×10 -11 M/L, as well as reusability via photocatalytic degrading the probe molecules, resulting in achieving recyclable SERS sensing applications. Furtherly, the outstanding SERS performance of the composite is demonstrated by recycling detection-degradation process for different molecules with acceptable performance decline. These results indicate that the Ag@AgCl@g-C 3 N 4 composite provides a new path for improving traditional single-use SERS substrates and promotes practical SERS applications in sustainable detection and removal of organic pollutants." @default.
• W4308463649 created "2022-11-12" @default.
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• W4308463649 date "2023-02-01" @default.
• W4308463649 modified "2023-10-05" @default.
• W4308463649 title "Plasmon-induced hot carrier separation across multicomponent heterostructure in Ag@AgCl@g-C3N4 composites for recyclable detection-removal of organic pollutions via SERS sensing" @default.
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• W4308463649 doi "https://doi.org/10.1016/j.apsusc.2022.155604" @default.
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