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- W4308482093 abstract "Despite tremendous investigations, a quantum spin liquid (QSL) state realized in a spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite $mathrm{Zn}{mathrm{Cu}}_{3}{(mathrm{O}mathrm{H})}_{6}{mathrm{Cl}}_{2}$, a quantum spin liquid candidate on the perfect kagome lattice, precisely characterizing the intrinsic physics of the kagome layers is extremely challenging due to the presence of interlayer Cu/Zn antisite disorder within its crystal structure. Here we measured the specific heat and thermal conductivity of single-crystal herbertsmithite in magnetic fields with high resolution. Strikingly, intrinsic magnetic specific heat contribution arising from the kagome layers exhibits excellent scaling collapse as a function of $T/H$ (temperature/magnetic field). In addition, no residual linear term in the thermal conductivity $ensuremath{kappa}/T(Tensuremath{rightarrow}0)$ is observed in zero and applied magnetic fields, indicating the absence of itinerant gapless excitations. These results capture a new essential feature of the QSL state of the kagome layers; localized orphan spins are induced by exchange bond randomness, surrounded by a nonitinerant QSL." @default.
- W4308482093 created "2022-11-12" @default.
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- W4308482093 date "2022-11-03" @default.
- W4308482093 modified "2023-10-18" @default.
- W4308482093 title "Universal scaling of specific heat in the <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mi>S</mml:mi><mml:mo>=</mml:mo><mml:mfrac><mml:mn>1</mml:mn><mml:mn>2</mml:mn></mml:mfrac></mml:mrow></mml:math> quantum kagome antiferromagnet herbertsmithite" @default.
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- W4308482093 doi "https://doi.org/10.1103/physrevb.106.174406" @default.
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