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- W4308486821 abstract "Dry reforming of methane economically converts methane and carbon dioxide into syngas (hydrogen and carbon monoxide) but requires high energy and often suffers from catalyst instability. Here, a surface-modulation strategy is demonstrated via decorating in situ defects on isolated nickel (Ni) atoms over La2O3 for boosting light-driven dry reforming of methane activity. Atomically dispersed 0.5Ni/La2O3 achieves a hydrogen evolution rate of 170.9 mol gNi−1 h−1. The reactivity is mainly attributed to photogenerated electrons, which overcome the limitations of a purely thermal system. The in situ generation of oxygen vacancies increases the initial-stage reactivity, where oxygen vacancies act as electron traps to accelerate charge separation and promote the adsorption/activation of reactants. The 0.5Ni/La2O3 catalyst exhibits strong inhibition of carbon coking and is sintering resistant, benefiting from the synergy between in situ oxygen vacancies and isolated nickel atoms." @default.
- W4308486821 created "2022-11-12" @default.
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- W4308486821 date "2022-11-01" @default.
- W4308486821 modified "2023-10-16" @default.
- W4308486821 title "An in situ defect engineering approach for light-driven methane dry reforming over atomically distributed nickel" @default.
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- W4308486821 doi "https://doi.org/10.1016/j.xcrp.2022.101127" @default.
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