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- W4308486937 abstract "• Reaction enthalpies of the formation from halides were measured for the three tetrachlorocuprates. • Layer shift parameter was suggested for the sake of comparison of thermochemical data. • Increasing layers shift and reducing molar volume tends to lower formation enthalpy. Three different tetrachlorocuprates A 2 CuCl 4 containing 3-aminopropionic, 4-aminobutyric and 6-aminohexanoic acid cations in A-sublattice were synthesized. The temperatures of the decomposition onset for A 2 CuCl 4 were found to increase slightly with the aliphatic chain length in A cation. The standard reaction enthalpies for the formation from organic ammonium chloride and anhydrous copper (II) chloride at T = 298.15 K, Δ r H ° hal,298 (“hal” denotes the formation from the source halides), were determined by isoperibolic solution calorimetry. The layer shift parameter S was introduced for the sake of comparison of thermochemical and structural data. Both original and literature thermochemical data indicate that simultaneous increase in S and decrease in the molar volume, V mol , leads to a decrease in the Δ r H ° hal,298 ." @default.
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- W4308486937 date "2023-02-01" @default.
- W4308486937 modified "2023-10-16" @default.
- W4308486937 title "Thermochemistry of some amino acid-based layered copper chlorides" @default.
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- W4308486937 doi "https://doi.org/10.1016/j.jct.2022.106949" @default.
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