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• W4308487168 abstract "Employing hydrazine oxidation reaction (HzOR) to substitute oxygen evolution reaction (OER) has been regarded as a promising alternative to realize energy-saving hydrogen generation during water splitting. Herein, we introduce a combined experimental and theoretical investigation of zeolitic imidazolate framework-67 coupling with CoNiSe-3 (ZIF67@CoNiSe-3) as an efficient electrocatalyst towards both hydrogen evolution reaction (HER) and HzOR. The as-prepared ZIF67@CoNiSe-3 with nanoflower structure and highly porous ultrathin nanosheet arrays can endow advanced electrocatalytic properties for HER and HzOR. For instance, ZIF67@CoNiSe-3 demands a low overpotential of 49 mV to generate 10 mA·cm−2 with a small Tafel slope of 41.4 mV·dec-1 for HER, while it can also reach an ultrahigh current density of 400 mA cm−2 at 0.13 V vs reversible hydrogen electrode (RHE) with a small Tafel slope of 44.3 mV·dec-1 for HzOR. When using ZIF67@CoNiSe-3 as both cathode and anode in a two-electrode cell for overall hydrazine splitting (OHzS), it only needs an ultralow cell voltage of 0.45 V to produce 100 mA·cm−2 with a remarkable long-term stability of 30 h. Impressively, first-principles calculations (DFT) have been employed to investigate the electrocatalytic mechanisms of ZIF67@CoNi-3 for HER and HzOR. This research could provide an efficient strategy for energy-saving H2 production during water splitting by incorporating a low-cost yet high-performance bifunctional catalyst." @default.
• W4308487168 created "2022-11-12" @default.
• W4308487168 creator A5059896405 @default.
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• W4308487168 date "2023-01-01" @default.
• W4308487168 modified "2023-10-14" @default.
• W4308487168 title "Bifunctional zeolitic imidazolate framework-67 coupling with CoNiSe electrocatalyst for efficient hydrazine-assisted water splitting" @default.
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• W4308487168 doi "https://doi.org/10.1016/j.jcis.2022.10.152" @default.
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