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- W4308489932 abstract "Developing efficient photosensitizers for C–P bond construction is highly important and remains a challenge due to the urgently needed for the synthesis of modified nucleosides, nucleotides, and other phosphine-containing ligands. Herein, two pyrene-tethered bismoviologen derivatives (Py-BiV2+) were designed and synthesized for visible-light-induced C–P bonds formation. The photochemical and electrochemical properties of Py-BiV2+ were studied systemically, certifying fine-tunable opto-electronic properties through the number of pyrene groups (4, n = 1; 6, n = 2). The prepared Py-BiV2+ showed strong light absorption, while retaining good redox features and chromic response features that were inherent to viologens. 4 exhibited accelerated photoinduced electron transfer in the presence of the electron donor (pyrene) and the generated 4′ (radical cation) showed higher stability. Accordingly, Py-BiV2+ directly served as photosensitizers for the first time in the visible-light-induced C(sp3)–P and C(sp2)–P bonds formation. As expected, these novel viologen derivatives exhibited good catalytic performance and good substrate expansibility under ambient conditions." @default.
- W4308489932 created "2022-11-12" @default.
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- W4308489932 date "2023-06-01" @default.
- W4308489932 modified "2023-10-03" @default.
- W4308489932 title "Pyrene-tethered bismoviologens for visible light-induced C(sp3)–P and C(sp2)–P bonds formation" @default.
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- W4308489932 doi "https://doi.org/10.1016/j.cclet.2022.107958" @default.
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