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- W4308499739 abstract "Green production process of high value-added bio-platform compounds is appealing yet challenging due to low catalyst performance and demand for acid or alkali conditions. Herein, we fabricated a tailored bio-tar derived super porous carbon material supported nano Pt catalyst via tuning the alkalinity by nitrogen doping. This novel catalyst realized an enhanced catalytic performance in selective oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-furandicarboxylic acid (FDCA) in alkaline free conditions, in which 97.8% HMF conversion and 54.7% FDCA selectivity were achieved under mild temperature (90 °C). The kinetic study revealed that the process is multi-step parallel reactions of 2,5-diformylfuran (DFF) and 5-formylfuran-2-carboxylic acid (FFCA) as intermediates from HMF, and the oxidation of carbonyl group in FFCA is the rate-determining step. This work provides a new synthesis method of low-cost catalyst by using organic waste and inspires a sustainable process for bio-platform compounds production with significant environmental benefits." @default.
- W4308499739 created "2022-11-12" @default.
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- W4308499739 date "2023-02-01" @default.
- W4308499739 modified "2023-10-15" @default.
- W4308499739 title "Pt/N co-doped porous carbon derived from bio-tar: A remarkable catalyst for efficient oxidation of 5-hydroxymethylfurfural under alkali-free condition: Performance, mechanism and kinetics" @default.
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- W4308499739 doi "https://doi.org/10.1016/j.cej.2022.140179" @default.
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