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- W4308581305 abstract "• The R sheet of PEDOT:PSS was significantly reduced with the Brij C10 additive. • Brij C10 markedly modified the electronic structure of a PEDOT:PSS surface. • XPS analysis indicates the increased relative ratio of conducting PEDOT. • An efficient charge transport pathway in PEDOT:PSS was formed. • The PCE of PSCs with a Brij C10-modified PEDOT:PSS anode was increased. The development of efficient transparent conducting electrodes (TCEs) is of great importance for achieving high-performance optoelectronic devices. Poly(3,4-ethylenedioxythiophene)-poly(styrene sulfonate) (PEDOT:PSS) is a well-known conducting polymer used in a wide range of applications. However, for electrode applications, the sheet resistance (R sheet ) of PEDOT:PSS must be significantly reduced to replace conventional TCEs. In this study, we demonstrated a significant decrease in R sheet of a PEDOT:PSS film by mixing polyethylene glycol hexadecyl ether (Brij C10) into the PEDOT:PSS solution. The electronic structure modified by the rearrangement of conducting PEDOT and insulating PSS with Brij C10 was investigated using X-ray photoelectron spectroscopy. The Brij C10 additive altered the interaction between PEDOT and PSS, and the relative ratio of conducting PEDOT on the film surface increased, thereby facilitating efficient charge transport. Using the reduced R sheet , perovskite solar cells (PSCs) with a Brij C10-modified PEDOT:PSS anode were fabricated. The power conversion efficiency of the PSCs was remarkably improved by reducing R sheet , indicating the high potential of the PEDOT:PSS electrode." @default.
- W4308581305 created "2022-11-12" @default.
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- W4308581305 date "2023-02-01" @default.
- W4308581305 modified "2023-10-14" @default.
- W4308581305 title "Electronic structure modification of polymeric PEDOT:PSS electrodes using the nonionic surfactant Brij C10 additive for significant sheet resistance reduction" @default.
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- W4308581305 doi "https://doi.org/10.1016/j.apsusc.2022.155609" @default.
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