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• W4308583235 abstract "The rapid deactivation of cost-effective MnO 2 -based catalysts in humid air limits their application in practical, and identification of the role of water in an oxidation process is significant for developing water-resistant MnO 2 -based catalysts. Here, CuMnO 2 showed 20.3% HCHO conversion in 10 h at room temperature in humid air with relative humidity of 40%, but deactivated in 3 h in dry air. The excellent activity and stability of HCHO oxidation in humid air were attributed to the positive effect of H 2 O on HCHO oxidation to the H 2 O-HOCH 2 OH supermolecule assemblies via hydrogen bonds formed on CuMnO 2 . H 2 O-HOCH 2 OH supermolecule assemblies tend to be oxidized to carbonate, which is further oxidized to CO 2 . Furthermore, CuMnO 2 exhibited a much poorer activity of CO oxidation in humid air, but the CO conversion was still 100% in 10 h in dry air. H 2 O showed a competitive adsorption effect to CO on CuMnO 2 . CuMnO 2 could be applied in HCHO elimination in humid air and CO elimination in dry air." @default.
• W4308583235 created "2022-11-12" @default.
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• W4308583235 date "2024-03-01" @default.
• W4308583235 modified "2023-10-12" @default.
• W4308583235 title "Investigation into the roles of interfacial H2O structure in catalytic oxidation of HCHO and CO over CuMnO2 catalysts" @default.
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• W4308583235 doi "https://doi.org/10.1016/j.jes.2022.10.044" @default.
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