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- W4308603206 abstract "The primary challenge for n-type small-molecule organic electrochemical transistors (OECTs) is to improve their electron mobilities and thus the key figure of merit μC *. Nevertheless, few reports in OECTs have specially proposed to address this issue. Herein, we report a 10-ring-fused polycyclic π-system consisting of the core of naphthalene bis-isatin dimer and the terminal moieties of rhodamine, which features intramolecular noncovalent interactions, high π-delocalization and strong electron-deficient characteristics. We find that this extended π-conjugated system using the ring fusion strategy displays improved electron mobilities up to 0.043 cm 2 V −1 s −1 compared to our previously reported small molecule gNR, and thereby leads to a remarkable μC * of 10.3 F cm −1 V −1 s −1 in n-type OECTs, which is the highest value reported to date for small-molecule OECTs. This work highlights the importance of π-conjugation extension in polycyclic-fused molecules for enhancing the performance of n-type small-molecule OECTs." @default.
- W4308603206 created "2022-11-13" @default.
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- W4308603206 date "2022-12-01" @default.
- W4308603206 modified "2023-10-16" @default.
- W4308603206 title "Electron‐Deficient Polycyclic Molecules via Ring Fusion for n‐Type Organic Electrochemical Transistors" @default.
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- W4308603206 doi "https://doi.org/10.1002/ange.202213737" @default.
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