Matches in SemOpenAlex for { <https://semopenalex.org/work/W4308616716> ?p ?o ?g. }
- W4308616716 endingPage "130366" @default.
- W4308616716 startingPage "130366" @default.
- W4308616716 abstract "As promising visible-light-responsive photocatalysts, triazine-based covalent organic frameworks (CTFs) still suffer from broad bandgap and high electron-hole recombination. As such, different contents of electron-rich ketone group were introduced to CTFs (X % keto-CTF), aiming to clarify the mechanism of quantitatively regulating ketone for enhanced visible-light photocatalytic performance of CTFs. As ketone content increased, the bandgap narrowed, electron-hole recombination decreased, charge transfer and quantum yield increased. As a result, keto-CTF outperformed other keto-CTFs in visible-light photocatalytic degradation of tetracycline, and apparent rate constant of TC (kobs) was 3.69 times higher than that of CTF. Importantly, ketone tuning induced varied types and concentrations of reactive species. Integrated with quantitative structure-activity relationships (QSARs) analysis and density functional theory (DFT) calculations, this study unravels how ketone content regulates bandgap structure of CTF, affects the contribution of varied reactive species, and quantitatively enhances the photocatalytic performance of CTFs. It also provides novel insights into the precise design and synthesis of CTFs-based catalyst structures for high-efficient visible-light photocatalytic degradation of organic pollutants." @default.
- W4308616716 created "2022-11-13" @default.
- W4308616716 creator A5039266973 @default.
- W4308616716 creator A5044757881 @default.
- W4308616716 creator A5048111390 @default.
- W4308616716 creator A5052753409 @default.
- W4308616716 creator A5056716586 @default.
- W4308616716 date "2023-02-01" @default.
- W4308616716 modified "2023-09-30" @default.
- W4308616716 title "Quantitatively regulating the ketone structure of triazine-based covalent organic frameworks for efficient visible-light photocatalytic degradation of organic pollutants: Tunable performance and mechanisms" @default.
- W4308616716 cites W1572819095 @default.
- W4308616716 cites W1973357647 @default.
- W4308616716 cites W1981368803 @default.
- W4308616716 cites W2029667189 @default.
- W4308616716 cites W2051982306 @default.
- W4308616716 cites W2055153070 @default.
- W4308616716 cites W2096747776 @default.
- W4308616716 cites W2116871840 @default.
- W4308616716 cites W2132525235 @default.
- W4308616716 cites W2155178633 @default.
- W4308616716 cites W2211450268 @default.
- W4308616716 cites W2236556070 @default.
- W4308616716 cites W2253772638 @default.
- W4308616716 cites W2262193673 @default.
- W4308616716 cites W2617038631 @default.
- W4308616716 cites W2622683700 @default.
- W4308616716 cites W2729037752 @default.
- W4308616716 cites W2739329531 @default.
- W4308616716 cites W2740266477 @default.
- W4308616716 cites W2749926733 @default.
- W4308616716 cites W2782678818 @default.
- W4308616716 cites W2792110135 @default.
- W4308616716 cites W2793040244 @default.
- W4308616716 cites W2795057659 @default.
- W4308616716 cites W2883275604 @default.
- W4308616716 cites W2885340048 @default.
- W4308616716 cites W2902920497 @default.
- W4308616716 cites W2942909499 @default.
- W4308616716 cites W2946049526 @default.
- W4308616716 cites W2948440280 @default.
- W4308616716 cites W2953544815 @default.
- W4308616716 cites W2961641437 @default.
- W4308616716 cites W2964732667 @default.
- W4308616716 cites W2970506507 @default.
- W4308616716 cites W2971712275 @default.
- W4308616716 cites W2972425990 @default.
- W4308616716 cites W2972511651 @default.
- W4308616716 cites W2975793409 @default.
- W4308616716 cites W2979795026 @default.
- W4308616716 cites W2980595943 @default.
- W4308616716 cites W2995688716 @default.
- W4308616716 cites W2997430076 @default.
- W4308616716 cites W3007687801 @default.
- W4308616716 cites W3013354084 @default.
- W4308616716 cites W3015607306 @default.
- W4308616716 cites W3015631441 @default.
- W4308616716 cites W3017101350 @default.
- W4308616716 cites W3017143397 @default.
- W4308616716 cites W3020591406 @default.
- W4308616716 cites W3025455773 @default.
- W4308616716 cites W3036316209 @default.
- W4308616716 cites W3082221893 @default.
- W4308616716 cites W3082868896 @default.
- W4308616716 cites W3083529509 @default.
- W4308616716 cites W3085308045 @default.
- W4308616716 cites W3109422539 @default.
- W4308616716 cites W3110452228 @default.
- W4308616716 cites W3127452237 @default.
- W4308616716 cites W3137165107 @default.
- W4308616716 cites W3138581249 @default.
- W4308616716 cites W3163328613 @default.
- W4308616716 cites W3194391130 @default.
- W4308616716 cites W3198640502 @default.
- W4308616716 cites W3207084205 @default.
- W4308616716 cites W3208575713 @default.
- W4308616716 cites W3213989100 @default.
- W4308616716 cites W4220821300 @default.
- W4308616716 doi "https://doi.org/10.1016/j.jhazmat.2022.130366" @default.
- W4308616716 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36434920" @default.
- W4308616716 hasPublicationYear "2023" @default.
- W4308616716 type Work @default.
- W4308616716 citedByCount "5" @default.
- W4308616716 countsByYear W43086167162023 @default.
- W4308616716 crossrefType "journal-article" @default.
- W4308616716 hasAuthorship W4308616716A5039266973 @default.
- W4308616716 hasAuthorship W4308616716A5044757881 @default.
- W4308616716 hasAuthorship W4308616716A5048111390 @default.
- W4308616716 hasAuthorship W4308616716A5052753409 @default.
- W4308616716 hasAuthorship W4308616716A5056716586 @default.
- W4308616716 hasConcept C104663316 @default.
- W4308616716 hasConcept C127413603 @default.
- W4308616716 hasConcept C147597530 @default.
- W4308616716 hasConcept C152365726 @default.
- W4308616716 hasConcept C161790260 @default.
- W4308616716 hasConcept C178790620 @default.
- W4308616716 hasConcept C180577832 @default.
- W4308616716 hasConcept C181966813 @default.
- W4308616716 hasConcept C185592680 @default.