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• W4308657925 abstract "Using ultrahigh magnetic field up to 120 T, a 1/2 magnetization plateau within $11.7--34.8$ T and a 3/4-like plateau within $55.6--87.0$ T have been observed in the $S$-1 skew chain antiferromagnet ${mathrm{Ni}}_{2}{mathrm{V}}_{2}{mathrm{O}}_{7}$. By combining density functional theory calculations, exact diagonalization, and quantum Monte Carlo simulations, we find that the nearest-neighbor interchain interaction (${J}_{3}/{k}_{text{B}}=ensuremath{-}78.5$ K) is much stronger than the intrachain interactions (${J}_{1}/{k}_{text{B}}=ensuremath{-}1.0$ K and ${J}_{2}/{k}_{text{B}}=6.3$ K), showing surprising ``dimerization'' of magnetic ions caused by the large $3d$-orbital overlap along the Ni1-Ni1 bond. Thus a ``$text{dimer}+text{monomer}$'' model is proposed to describe the magnetization process---the 1/2 plateau pertains to weakly coupled Ni2 monomers while the 3/4-like plateau to the strongly coupled Ni1 dimers. The possible supersolid phases from the Ni1 dimers are proposed." @default.
• W4308657925 created "2022-11-13" @default.
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• W4308657925 date "2022-11-09" @default.
• W4308657925 modified "2023-10-18" @default.
• W4308657925 title "Unusual dimerization and magnetization plateaus in <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mi>S</mml:mi></mml:mrow></mml:math> = 1 skew chain <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>Ni</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>V</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>7</mml:mn></mml:msub></mml:mrow></mml:math> observed at 120 T" @default.
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• W4308657925 doi "https://doi.org/10.1103/physrevb.106.184409" @default.
• W4308657925 hasPublicationYear "2022" @default.
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