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• W4308746319 endingPage "155631" @default.
• W4308746319 startingPage "155631" @default.
• W4308746319 abstract "The honeycomb-like porous carbon incorporated with CdS/ZnS heterojunction for TC degradation and H 2 generation has been successfully fabricated by an easy-handling calcination route. • 1. A simple and novel strategy was proposed to construct CdS/ZnS heterojunction loaded on honeycomb-like porous carbon (CZS@C). • 2. CZS@C showed excellent visible-light-driven photocatalytic activity towards TC degradation and H 2 generation. • 3. Mechanism and pathways for the TC degradation and H 2 generation were discussed in details. • 4. The photocatalyst exhibited the outstanding stability and reusability. Accelerating the charge separation efficiency is a crucial approach to improve the photocatalytic performance of semiconductors. The design and synthesis of heterojunctions can effectively inhibit the recombination of photogenerated electron-hole pairs and enhance the charge separation efficiency. In this work, an easy-handling calcination route was proposed to prepare CdS/ZnS heterojunction loaded on honeycomb-like porous carbon (CZS@C) using chitosan as a precursor. The unique honeycomb-like porous structure facilitated the separation and migration of photoexcited electrons and holes, improving the utilization of visible light and shortening the distance of electron transport. The photocatalytic performance of CZS@C was evaluated by the degradation of tetracycline (TC) and H 2 production from water splitting under visible light. The optimized CZS@C composite can degrade almost 92.40% of TC under visible light irradiation in 60 min. Such CZS@C composite presented an excellent photocatalytic activity with H 2 production rate of 5.49 mmol h -1 g -1 , which was 54.9 and 2.28-folds higher than ZnS@C and CdS@C. Furthermore, the possible photocatalytic reaction mechanism and pathway towards TC degradation and simultaneous H 2 generation was proposed." @default.
• W4308746319 created "2022-11-15" @default.
• W4308746319 creator A5012429068 @default.
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• W4308746319 date "2023-02-01" @default.
• W4308746319 modified "2023-10-16" @default.
• W4308746319 title "Honeycomb-like porous carbon loaded with CdS/ZnS heterojunction with enhanced photocatalytic performance towards tetracycline degradation and H2 generation" @default.
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• W4308746319 doi "https://doi.org/10.1016/j.apsusc.2022.155631" @default.
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