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• W4308834850 abstract "Hydrodynamic chromatography (HDC) is a well-established analytical separation method for the size separation of nano- and microparticles and large molecular weight solutes such as synthetic polymers and proteins. We report on a theoretical study showing that the separation resolution of open-tubular HDC can be significantly enhanced by changing the cross-sectional shape of the separation channel. By enforcing Brenner’s macro-transport approach, we provide theoretical/numerical evidence showing how the shape of the cross section influences quantitatively both the selectivity and the axial dispersion of the suspended particles in HDC. The separation performance of square-, triangle-, and star-shaped channel cross sections is compared to that of a cylindrical capillary over three decades of the particle Péclet number in terms of the minimal separation length and time to obtain the unit resolution of a two-particle mixture. Enhancement factors up to 400% are found in the case of triangular shapes, with the best performing case being the 70.6° angle, which can be obtained by KOH etching of bulk silicon." @default.
• W4308834850 created "2022-11-17" @default.
• W4308834850 creator A5015646507 @default.
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• W4308834850 date "2022-11-12" @default.
• W4308834850 modified "2023-10-01" @default.
• W4308834850 title "Shape-Enhanced Open-Channel Hydrodynamic Chromatography" @default.
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• W4308834850 doi "https://doi.org/10.1021/acs.analchem.2c02766" @default.
• W4308834850 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36370088" @default.
• W4308834850 hasPublicationYear "2022" @default.
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