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• W4308953901 abstract "Although perovskite wafers with a scalable size and thickness are suitable for direct X-ray detection, polycrystalline perovskite wafers have drawbacks such as the high defect density, defective grain boundaries, and low crystallinity. Herein, PbI2 -DMSO powders are introduced into the MAPbI3 wafer to facilitate crystal growth. The PbI2 powders absorb a certain amount of DMSO to form the PbI2 -DMSO powders and PbI2 -DMSO is converted back into PbI2 under heating while releasing DMSO vapor. During isostatic pressing of the MAPbI3 wafer with the PbI2 -DMSO solid additive, the released DMSO vapor facilitates in situ growth in the MAPbI3 wafer with enhanced crystallinity and reduced defect density. A dense and compact MAPbI3 wafer with a high mobility-lifetime (µτ) product of 8.70 × 10-4 cm2 V-1 is produced. The MAPbI3 -based direct X-ray detector fabricated for demonstration shows a high sensitivity of 1.58 × 104 µC Gyair-1 cm-2 and a low detection limit of 410 nGyair s-1 ." @default.
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• W4308953901 date "2022-11-13" @default.
• W4308953901 modified "2023-10-18" @default.
• W4308953901 title "PbI₂‐DMSO Assisted In Situ Growth of Perovskite Wafers for Sensitive Direct X‐Ray Detection" @default.
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• W4308953901 doi "https://doi.org/10.1002/advs.202204512" @default.
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