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- W4308954845 abstract "Due to the very distinct electronic band structure and lower power factor, the exploration of n-type PbTe as thermoelectric materials has historically fallen behind that of p-type PbTe. In this work, n-type Pb0.97Sb0.03Te-based composites incorporated with Cu12Sb4S13 nanoparticles are synthesized and investigated. Sb doping is utilized to modify its carrier concentration in order to obtain n-type PbTe materials with a high power factor. Then, the incorporation of Cu12Sb4S13 nanoparticles can generate semi-coherent nanophase CuTe, and simultaneously optimize the thermal and electrical properties due to remarkable energy filtering effects and interface scattering in the higher temperature range. Eventually, a peak figure of merit ZT ≈ 1.58 was obtained at 773 K for the sample Pb0.97Sb0.03Te + 1.5 wt% Cu12Sb4S13, indicating that the incorporation of Cu12Sb4S13 in Pb0.97Sb0.03Te is an effective approach to improve its thermoelectric performance." @default.
- W4308954845 created "2022-11-20" @default.
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- W4308954845 date "2022-01-01" @default.
- W4308954845 modified "2023-10-16" @default.
- W4308954845 title "Achieving higher thermoelectric performance of n-type PbTe by adjusting the band structure and enhanced phonon scattering" @default.
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- W4308954845 doi "https://doi.org/10.1039/d2nr04419f" @default.
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