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- W4308978897 abstract "Monazite-cheralite ceramics are a promising waste form for actinides. To elucidate the long-term behavior of this matrix in aqueous solutions, this study measured thermodynamic data for Th-rhabdophanes Ln1-2xCaxThxPO4·nH2O (with Ln = Pr, Nd; x = 0–0.15) and the associated anhydrous monazite-cheralites Ln1-2xCaxThxPO4. Solubility experiments at 298 K and high temperature oxide melt solution calorimetry were combined for calculation of ΔGf°, ΔHf° and Sm° of Th-rhabdophanes and associated monazite-cheralites. Standard solubility constants were employed in a geochemical simulation using the PHREEQC software, the results of which confirmed the high chemical stability of the monazite-cheralite phases and supported their use as a specific conditioning matrix for the long-term immobilization of actinides." @default.
- W4308978897 created "2022-11-20" @default.
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- W4308978897 date "2023-01-01" @default.
- W4308978897 modified "2023-10-14" @default.
- W4308978897 title "Chemical and environmental stability of monazite-cheralite solid solutions Ln1-2Ca Th PO4 (Ln = Pr, Nd; x = 0–0.15): A thermodynamic study" @default.
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- W4308978897 doi "https://doi.org/10.1016/j.apgeochem.2022.105504" @default.
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