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• W4308991110 startingPage "18842" @default.
• W4308991110 abstract "We have prepared a series of complexes of the type [IrIII(ppy)2(L]n+ complexes (1–4), where ppy is a substituted 2-phenylpyridine and L is a chelating phosphine thioether ligand. The parent complex (1) comprises an unsubstituted phenylpyridine ligand, whereas complex 2 contains a nitro substituent on the pyridine ring, complex 3 features a diphenylamine group on the phenyl ring, and 4 has both nitro and diphenylamine groups. Crystallographic, 1H NMR, and elemental analysis data are consistent with each of the chemical formulae. DFT (density functional theory) computational results show a complicated electronic structure with contributions from Ir, ppy, and the PS ligand. Ultrafast pump–probe data show strong contributions from the phenylpyridine moieties as well as strong panchromatic excited state absorption transitions. The data show that nitro and/or diphenylamine substituents dominate the spectroscopy of this series of compounds." @default.
• W4308991110 created "2022-11-20" @default.
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• W4308991110 date "2022-11-14" @default.
• W4308991110 modified "2023-10-15" @default.
• W4308991110 title "Manipulating Excited State Properties of Iridium Phenylpyridine Complexes with “Push–Pull” Substituents" @default.
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• W4308991110 doi "https://doi.org/10.1021/acs.inorgchem.2c02269" @default.
• W4308991110 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36375136" @default.
• W4308991110 hasPublicationYear "2022" @default.
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