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- W4309078918 abstract "Anode-free lithium metal batteries (AFLMBs) can achieve a high energy density. However, achieving high-capacity retention and Coulombic efficiency (CE) are challenging without a continuous Li supply from the Cu anode side. The lower CE and rapid capacity decay in AFLMBs are primarily due to non-uniform Li deposition and electrolyte decomposition during cycling. Herein, strontium fluoride (SrF2) nanoparticles are applied on Cu foils to attain the in-situ forming of a bifunctional interfacial layer, a Li-Sr alloy, and a LiF-rich SEI composite layer during Li plating. The derived [email protected]2 electrode has excellent plating/stripping stability and outstanding performance. AFLMB full cell ([email protected]2//NCM111) attains an average Coulombic efficiency (ACE) of 98.6 % and capacity retention of 51.0 % at the 60th cycle using a commercial carbonate-based electrolyte. In contrast, the bare AFLMB full cell (BCu//NCM111) only has an ACE of 94.9 % with a capacity retention of 10.2 % under the same conditions. The concept is proven in lithium metal batteries (LMBs). This strategy provides a simultaneous Li nucleation and formation of LiF-rich SEI layers, rendering it promising to realize AFLMBs and LMBs with long lifespans and high CE." @default.
- W4309078918 created "2022-11-21" @default.
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- W4309078918 date "2022-12-01" @default.
- W4309078918 modified "2023-10-17" @default.
- W4309078918 title "An in-situ formed bifunctional layer for suppressing Li dendrite growth and stabilizing the solid electrolyte interphase layer of anode free lithium metal batteries" @default.
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- W4309078918 doi "https://doi.org/10.1016/j.est.2022.105955" @default.
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