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- W4309101394 abstract "• Blisters are observed in Au sputter-coating on Ni-based single crystal superalloy. • Their diameters increase, but diameter-to-height ratios don’t, with film thickness. • They prefer to form on the γ-matrix rather than the γ′-precipitate or Si substrate. • DFT calculations indicate a higher tendency of moisture adsorption on γ than on γ′ • Mechanical modelling shows blistering is driven by pocket of energy concentration. Au thin films, up to h ≈ 90 nm thick, have been deposited by direct current sputtering at room temperature to address the effect of coating thickness on film blistering that occurred on Ni-based single crystal (NBSC) superalloy rather than on Si. Transmission electron microscopy provides evidence that the blisters nucleated at the Au/NBSC interface. Statistically, the diameters of the blisters increases while their density decreases with the increase in h ; however, the height-to-diameter ratios of the blisters measured from the film surface are rather constant and independent of h . When h is increased from ≤ 63 nm to ∼90 nm, the size distribution of the blisters turns from a single mode to a bimodal along with an emergence of larger circular blisters and edge-like ones. Mechanical modelling and density-function calculations provide evidence that the formation of blisters is driven by pockets of energy concentration while the nucleation site is influenced by surface absorbents of the substrate." @default.
- W4309101394 created "2022-11-22" @default.
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- W4309101394 date "2023-02-01" @default.
- W4309101394 modified "2023-09-27" @default.
- W4309101394 title "Insights into thin film blistering of gold coating on metal substrate" @default.
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- W4309101394 doi "https://doi.org/10.1016/j.apsusc.2022.155700" @default.
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