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- W4309147519 endingPage "126713" @default.
- W4309147519 startingPage "126713" @default.
- W4309147519 abstract "• A novel Fe-doped cobalt-based metal organic frameworks was prepared by a one-step method. • Co/Fe-MOF was used to uptake SeO 3 2- , and the maximum adsorption capacity was 283.11 mg g −1 of Co-MOF. • Under the condition of sacrificing a small amount of adsorption capacity, Co 0.90 Fe 0.10 -MOF can be used in the broader pH range with higher stability. • U-Co/Fe were recycled utilization as an OER electrocatalyst in wastewater treatment process. As the main form exists in selenium-containing wastewater, selenite (SeO 3 2- ) is often produced by human activities and is exceedingly difficult to be removed from wastewater. In this study, five iron-doped (Fe-doped) cobalt-based metal organic frameworks (Co/Fe-MOF) with different metal ratios were prepared to remove SeO 3 2- anions. The prepared Co/Fe-MOF were confirmed by characterization and their adsorption properties experiments. They have excellent SeO 3 2- removal performance at pH of 3–8 with a maximum adsorption capacity of 283.11 mg g −1 of Co-MOF. After uptaking SeO 3 2- by Co/Fe-MOF, the used Co/Fe-MOF (U-Co/Fe) contains CoSeO 4 and Fe 2 (SeO 4 ) 3 and can be used as electrocatalytic oxygen evolution catalysts. Their oxygen/selenium vacancies can reduce the overpotential of the oxygen evolution reaction (OER). In 1.0 M KOH, U-Co 0.90 Fe 0.10 displayed the lowest overpotential 326 mV at 10 mA cm −2 . This study reveals the mechanism and resource upgrading process of SeO 3 2- removal by Co/Fe-MOF and demonstrates that a small amount of Fe doping could improve the performance of OER." @default.
- W4309147519 created "2022-11-23" @default.
- W4309147519 creator A5005249136 @default.
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- W4309147519 date "2023-02-01" @default.
- W4309147519 modified "2023-09-26" @default.
- W4309147519 title "Removal and recycling of selenite anions by iron-doped cobalt-based metal organic frameworks for oxygen evolution reaction" @default.
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- W4309147519 doi "https://doi.org/10.1016/j.fuel.2022.126713" @default.
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