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• W4309261746 endingPage "126781" @default.
• W4309261746 startingPage "126781" @default.
• W4309261746 abstract "• Hydrogen increases by 18.48% from poplar pyrolysis on iron-based aluminum dross. • Iron-based aluminum dross enhances three-dimensional diffusion for hydrogen generation. • Tar condensation on 200AD-6 %Fe forms higher phenols for promoting hydrogen production. • C O M complexes with more condensation of aromatic units improve hydrogen production. Iron based on aluminum dross was prepared to enhance hydrogen production by impregnated method. The pyrolysis experiments are performed in a fix-bed reactor to obtain pyrolysis product distribution. The pyrolysis behavior of poplar on iron-based aluminum dross was studied by thermogravimetric analysis (TG), and hydrogen composition in pyrolysis gas were determined by gas chromatography (GC). The results show that iron-based aluminum dross has a significant effect on improving hydrogen generation. The iron-based aluminum dross with 6% iron on aluminum dross promotes hydrogen by 18.48% compared with poplar. The kinetic calculation shows that the activation energy increases by 20.53% at conversion rate of 0.8, indicating that iron-based aluminum dross increases the condensation reaction degree with the pyrolysis residue increasing and requires more external energy for bond dissociation at high-temperature stage. Hydrogen generation is dominated by contracting volume and diffusional theory controlled by Carbon-Oxygen-Metal (C O M) active intermediate during pyrolysis on iron-based aluminum dross. Pyrolysis reactivity of poplar is improved during the reaction of A1-A4 nucleation and growth stage in low-temperature stage. The high-temperature stage follows the F3 and D3 models and the gas diffusion rate increases to enhance active intermediate generation for hydrogen production." @default.
• W4309261746 created "2022-11-25" @default.
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• W4309261746 date "2023-02-01" @default.
• W4309261746 modified "2023-10-04" @default.
• W4309261746 title "Pyrolysis of wood waste to enhance hydrogen production on iron-based aluminum dross" @default.
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• W4309261746 doi "https://doi.org/10.1016/j.fuel.2022.126781" @default.
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