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- W4309279564 abstract "The selectivity filter of biological ion channels could well split ion’s hydration shell at the entryway of channels with subtle opening sizes, leading to the ‘naked’ ion’s rapid transport across the channels. Numerous artificial nanochannels have been developed for mimicking this. However, the precise fabrication of nanochannels/nanopores with targeted diameters has been always a challenge. Herein, we employ the immiscible liquid-infused channels to regulate the ion’s hydration shell and mimic the ion transport processes. Experimental and theoretical results show the partial removal of water molecules around ions at the entrance of the nanochannels and low-resistance migration of ions in the immiscible liquid phase. Compared with the pristine membrane, the cross-membrane conductance and osmotic energy power density of the proposed membrane have increased by ∼4-fold and ∼77.3%, respectively. Moreover, this approach avoids the far-reached technique and could be easily adapted to various membrane materials. Therefore, this strategy holds great potential in systems requiring ion transport across membranes, including ion separation, battery, and desalination, etc." @default.
- W4309279564 created "2022-11-25" @default.
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- W4309279564 date "2023-01-01" @default.
- W4309279564 modified "2023-10-17" @default.
- W4309279564 title "Immiscible liquid-mediated ultrafast ion transport through nanoconfined channels" @default.
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- W4309279564 doi "https://doi.org/10.1016/j.nanoen.2022.108011" @default.
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