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• W4309288514 endingPage "232346" @default.
• W4309288514 startingPage "232346" @default.
• W4309288514 abstract "High energy density and high-safety is expected for the ongoing revolution of lithium-ion batteries (LIBs). All-solid-state lithium metal batteries (ASSLMBs) are promising to break through the bottleneck of traditional liquid LIBs. However, the huge interfacial resistance between solid electrolytes and cathode is a hinder to the develop ASSLMBs. Herein, we report an in-situ polymerized solid-state electrolytes (SPE) based on oligomeric cyclotetrasiloxane (CTS) and polyethylene glycol diglycidyl ether (PEGDE) to solve this problem. CTS can provide a three-dimensional skeleton for the cross-linked SPE, which can effectively improve the properties of SPE. When the CTS content is 10 wt%, SPE exhibits a high ionic conductivity at 28 °C (0.37 mS cm−1) and a wide electrochemical stable window of 5.02 V (vs Li/Li+). Benefiting from the in-situ polymerization properties, ionic transportation at the cathode/electrolyte interface can be enhanced. Especially, the in-situ SPE exhibits outstanding compatibility against lithium metal over 600 h at a current density of 0.2 mA cm−2, the Li/SPE/LiCoO2 can deliver a capacity of 120.5 mAh g−1 at 0.05 C after 100 cycles. Our study, therefore, provides a new type of SPE to meet both interfacial and bulk conductivity requirements for ASSLMBs." @default.
• W4309288514 created "2022-11-25" @default.
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• W4309288514 date "2023-01-01" @default.
• W4309288514 modified "2023-10-18" @default.
• W4309288514 title "In-situ polymerized electrolyte modified with oligomeric cyclotetrasiloxane for all-solid-state lithium metal batteries" @default.
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• W4309288514 doi "https://doi.org/10.1016/j.jpowsour.2022.232346" @default.
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