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- W4309441707 abstract "Sequential energy transfer widely exists in natural light-harvesting systems (LHSs), which greatly benefits the full use of solar energy. In this work, we report an artificial light-harvesting platform derived from pillar (Wang et al., 2021) [5]arene-directed host-guest nanoparticles ( WP5 ⊃ G ) in aqueous media. The WP5 ⊃ G assembly can serve as a good donor owing to the excellent fluorescence behavior of G in the aggregated state, guaranteeing a two-step FRET from the WP5 ⊃ G to the relay acceptor eosin Y ( ESY ) and then to the final acceptor Nile red ( NiR ) to form a WP5 ⊃ G @ ESY / NiR system with high efficiency. As a consequence of the flexibility of the system, tunable emission including a highly efficient white-light emission can be realized. The WP5 ⊃ G @ ESY / NiR system was further used as a photocatalyst to catalyze dehalogenation reaction in aqueous solution, exhibiting remarkable catalytic activity as compared with the WP5 ⊃ G or ESY / NiR alone. • A light-harvesting system based on self-assembly was successfully fabricated. • The system contains a stepwise energy transfer process. • The material is color tunable and a bright white-light emission was realized. • The material can be used as a photocatalyst for dehalogenation reaction. • The fabrication and application of the system were totally in an aqueous media." @default.
- W4309441707 created "2022-11-27" @default.
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- W4309441707 date "2023-02-01" @default.
- W4309441707 modified "2023-09-29" @default.
- W4309441707 title "Pillar[5]arene-based light-harvesting assemblies with sequential energy-transfer for tunable emission and photocatalysis" @default.
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- W4309441707 doi "https://doi.org/10.1016/j.dyepig.2022.110958" @default.
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