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- W4309443054 abstract "Iron-based Prussian blue analogs (Fe-PBAs) are extensively studied as promising cathode materials for rechargeable sodium-ion batteries owing to their high theoretical capacity, low-cost and facile synthesis method. However, Fe-PBAs suffer poor cycle stability and low specific capacity due to the low crystallinity and irreversible phase transition during excess sodium-ion storage. Herein, a modified co-precipitation method to prepare highly crystallized PBAs is reported. By introducing an electrochemical inert element (Zn) to substitute the high-spin Fe in the Fe-PBAs (ZnFeHCF-2), the depth of charge/discharge is rationally controlled to form a highly reversible phase transition process for sustainable sodium-ion storage. Minor lattice distortion and highly reversible phase transition process of ZnFeHCF-2 during the sodium-ions insertion and extraction are proved by in-situ tests, which have significantly impacted the cycling stability. The ZnFeHCF-2 shows a remarkably enhanced cycling performance with capacity retention of 58.5% over 2000 cycles at 150 mA g−1 as well as superior rate performance up to 6000 mA g−1 (fast kinetics). Furthermore, the successful fabrication of the full cell on the as-prepared cathode and commercial hard carbon anode demonstrates their potential as high-performance electrode materials for large-scale energy storage systems." @default.
- W4309443054 created "2022-11-27" @default.
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- W4309443054 date "2022-11-20" @default.
- W4309443054 modified "2023-10-16" @default.
- W4309443054 title "Low‐Cost Zinc Substitution of Iron‐Based Prussian Blue Analogs as Long Lifespan Cathode Materials for Fast Charging Sodium‐Ion Batteries" @default.
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- W4309443054 doi "https://doi.org/10.1002/adfm.202210725" @default.
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