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- W4309485613 abstract "Effective strategies to improve charge separation in semiconductor particles are critical for improving the photodegradation of organic pollutants at levels sufficient for environmental applications. Herein, Bi2MoO6 (BMOMOF), comprising both nanoparticles (NPs) and quantum dots (QDs), was synthesized from a bismuth-based metal-organic framework (Bi-MOF) precursor. Surface defects on BMOMOF, the combination of NPs and QDs, and modified energy band edges improved photogenerated charge separation and facilitated redox reactions. When compared to BMO derived from uncoordinated Bi, the BMOMOF photocatalyst (PC) was more efficient at photodegrading tetracycline hydrochloride (TCH) and ciprofloxacin (CIP), two widely-used antibiotics ubiquitous in wastewater, as well as the carcinogenic pollutant rhodamine B (RhB). BMOMOF was then loaded on the biopolymer bacterial cellulose (BC) to further enhance photocatalytic performance and facilitate the recovery of the PC after water treatment processes. The novel BMOMOF/BC photocatalytic flakes were significantly larger than pure BMOMOF, and thus easier to recuperate. Furthermore, anchoring BMOMOF on BC flakes augmented significantly the photodegradation of TCH, CIP, and RhB, mainly because hydroxyl groups in BC act as hole traps facilitating photogenerated electron-hole separation. Results obtained with BMOMOF/BC highlight promising approaches to develop optimal PCs for aqueous pollutants degradation." @default.
- W4309485613 created "2022-11-28" @default.
- W4309485613 creator A5004314478 @default.
- W4309485613 creator A5005271698 @default.
- W4309485613 creator A5010058545 @default.
- W4309485613 creator A5026720737 @default.
- W4309485613 creator A5033510051 @default.
- W4309485613 creator A5043895973 @default.
- W4309485613 creator A5078166832 @default.
- W4309485613 date "2023-01-01" @default.
- W4309485613 modified "2023-10-07" @default.
- W4309485613 title "Bacterial cellulose flakes loaded with Bi2MoO6 nanoparticles and quantum dots for the photodegradation of antibiotic and dye pollutants" @default.
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