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- W4309487654 abstract "The design and construction of electrocatalysts with multiple components to modulate the intrinsic catalytic activity is a compelling strategy to achieve Pt-like activity for hydrogen generation. Challenging on the inert Cu-based electrocatalysts for water reduction, herein, a novel and fruitful CuRu-based electrocatalysts (RuCuOx/NC) is established by combining dual-templates assembling and pyrolysis protocol with a subsequent hot-alkali corrosion. Benefitting from the synergetic effect of Cu2+1O (with copper excess defects) and Ru, the as-prepared RuCuOx/NC affords brilliant activity and stability under alkaline condition. In 1 M KOH, the RuCuOx/NC provides Pt-like activity with overpotential of ∼29 mV to reach 10 mA cm−2. Theoretical calculations certified that H2O dissociation was accelerated and hydrogen adsorption free energy was optimized by the cooperation of Cu2+1O and Ru. This work proposes a promising methodology to construct multi-components electrocatalysts, which may lend perspective for the design of advanced electrocatalysts for renewable energy systems." @default.
- W4309487654 created "2022-11-28" @default.
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- W4309487654 date "2023-05-01" @default.
- W4309487654 modified "2023-09-25" @default.
- W4309487654 title "Cooperative hydrogen evolution reaction combining Cu2+1O and Ru active sites" @default.
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- W4309487654 doi "https://doi.org/10.1016/j.apcatb.2022.122169" @default.
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