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- W4309522664 abstract "The photoexcited free carrier dynamics in V2O5 microparticles are studied using time-resolved nondegenerate pump–probe transmission spectroscopy. By employing a numerically solved polaronic kinetic model on the time-resolved absorption obtained from transmission data, the self-trapping of free carriers, i.e., formation of polarons, and the self-trap assisted bimolecular decay in V2O5 microparticles are investigated. Also, by performing the fluence-dependent experiments, the variation of the various processes with the photoexcited carrier density is understood by invoking the carrier screening effect. It is estimated from this work that the average density of polarons is ∼2.58 × 1017cm–3, with their formation time of ∼4.5 ps." @default.
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- W4309522664 date "2022-11-21" @default.
- W4309522664 modified "2023-10-17" @default.
- W4309522664 title "Photoexcited Ultrafast Dynamics of Free Carriers and Polarons in V<sub>2</sub>O<sub>5</sub> Microparticles through Time-Resolved Nondegenerate Pump Probe Spectroscopy" @default.
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- W4309522664 doi "https://doi.org/10.1021/acs.jpcc.2c06894" @default.
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