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- W4309526101 abstract "Adsorption desulfurization is a very effective method to remove thiophenic compounds from fuels. The metal–organic frameworks (MOFs) have emerged as a new type of desulfurization adsorbents because of their porous nature and large specific surface area. In this study, Cu2+ was covalently introduced into the UiO-66 framework at the defective sites by the solvothermal method. Further, the π-complexation adsorbent UiO-66-Cu(I) containing Cu+ for adsorption desulfurization was synthesized by the methanol vapor-induced reduction. The adsorption performance was tested for the removal of thiophene from the model fuels with different sulfur concentrations. In comparison with the pristine UiO-66, the adsorbent UiO-66-Cu(I) has a higher adsorption capacity for thiophene, reaching 14.8 mg S/g. The competitive adsorption results indicated that UiO-66-Cu(I) has good selectivity for thiophene in the presence of aromatic compounds. From the recycling experiments, this adsorption still has the 86 % of the initial capacity after four cycles, indicating that the adsorbent has a good recycling performance." @default.
- W4309526101 created "2022-11-28" @default.
- W4309526101 creator A5005399281 @default.
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- W4309526101 date "2023-03-01" @default.
- W4309526101 modified "2023-10-18" @default.
- W4309526101 title "Construction of the π-complexation desulfurization adsorbent containing Cu+ at defective sites of UiO-66" @default.
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- W4309526101 doi "https://doi.org/10.1016/j.jiec.2022.11.041" @default.
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