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- W4309552904 abstract "K-doped FeC x catalysts derived from the carbothermal reduction of the Fe-chitosan complex were investigated and tested in the hydrogenation of CO 2 to light olefins (C 2-6 = ). Catalyst characterization, including bulk composition, porosity, crystallinity, Fe coordination, morphology, surface property, and basicity, was conducted. The physicochemical properties of tested catalysts were correlated with their performances. The mechanistic study discovered that bidentate carbonates, monodentate carbonate, bicarbonate, and formate species were intermediates involved in C 2-6 = synthesis. The yield of C 2-6 = was found to be dependent on the composition of the carbide phases of K-doped FeC x catalysts. The most active catalyst, i.e., FeK@CS-(0.5)-py, showed the most promising space-time yield of C 2-6 = (13.7 μmol C2-6= /g Fe /s). • K-doped FeC x catalysts were derived from the Fe-chitosan complexes. • A proper Fe-to-chitosan is important to increase the FeC x content. • A positive correlation between FeC x and the yield of C 2-6 = olefins was found. • Carbonates and formate were identified as the possible intermediates." @default.
- W4309552904 created "2022-11-28" @default.
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- W4309552904 date "2023-02-01" @default.
- W4309552904 modified "2023-10-14" @default.
- W4309552904 title "Catalytic hydrogenation of CO2 to light olefins by using K-doped FeCx catalysts derived from the Fe-chitosan complex" @default.
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- W4309552904 doi "https://doi.org/10.1016/j.ijhydene.2022.11.010" @default.
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