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- W4309553218 abstract "Membrane development in organic redox flow batteries (ORFBs) is of significant importance. Herein, we designed a series of anion exchange membranes made from poly(p-phenylene oxide) (PPO) with different degrees of functionalization, cationic moieties and crosslinking degrees. We tested them in a N,N,N-2,2,6,6-heptamethylpiperidinyl oxy-4-ammonium chloride/1,1′-dimethyl-4,4′-bipyridinium dichloride (TMA-TEMPO/MV) based ORFB single cell to investigate the structure-property-performance relationship. The common problem of active species crossover is solved by controlling the membrane water uptake below 70 wt.%, resulting in stable systems with coulombic efficiency of over 99.3%. The cell employing a membrane prepared from PPO and trimethylamine moiety attached via a C6-spacer achieved the best overall cell performance. It delivered high capacity retention (94% after over 100 consecutive cycles) and higher peak power density (293 mW·cm−2 at 16 mL·min−1) and energy efficiency (80%) than the commercial reference memane FAA-3-50." @default.
- W4309553218 created "2022-11-28" @default.
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- W4309553218 date "2023-01-01" @default.
- W4309553218 modified "2023-10-18" @default.
- W4309553218 title "Anion exchange membranes with high power density and energy efficiency for aqueous organic redox flow batteries" @default.
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- W4309553218 doi "https://doi.org/10.1016/j.electacta.2022.141565" @default.
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