FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4309631799> ?p ?o ?g. }

• W4309631799 endingPage "3900" @default.
• W4309631799 startingPage "3893" @default.
• W4309631799 abstract "Graphitic carbon nitride (GCN) has drawn widespread interests in solar hydrogen production. However, the difficult exfoliation and the intrinsic shortcomings greatly restrict the hydrogen production efficiency. Herein, we report a chlorine-mediated strategy to synthesize ultrathin wavy-structured GCN nanosheets for enhancing photocatalytic activity. Chlorine is firstly doped into the melem-based oligomer; in subsequent polymerization process, self-exfoliated wavy-structured GCN are obtained owing to the effect from chlorine removal. The obtained wavy-GCN presents superior H 2 evolution rate at 3372 μmol·g −1 h −1 , which is 25 times higher than pristine GCN. Comprehensive characterizations reveal two main reasons for the enhanced photocatalytic activity. 1) The GCN is in-situ self-exfoliated owing to removal of doped chlorine, increasing accessible active sites. 2) The introduction of nitrogen-defects into GCN gives rise to enhanced light absorption capacity and reduced charge carriers recombination rate. This work provides a new bottom-up two-step strategy for structural regulation of GCN towards enhanced photocatalytic performance. The two-step chlorine-regulated strategy to obtain ultrathin wavy-structured GCN for enhancing photocatalytic hydrogen production performance. • Providing a novel two-step strategy for exfoliation and structural regulation of GCN. • Obtaining the ultrathin wavy-structured GCN without extra exfoliation. • The obtained wavy-GCN with nitrogen-defects presents enhanced H 2 evolution rate." @default.
• W4309631799 created "2022-11-28" @default.
• W4309631799 creator A5003642180 @default.
• W4309631799 creator A5012985474 @default.
• W4309631799 creator A5061575283 @default.
• W4309631799 creator A5073188500 @default.
• W4309631799 creator A5076596665 @default.
• W4309631799 creator A5083125123 @default.
• W4309631799 date "2023-02-01" @default.
• W4309631799 modified "2023-10-17" @default.
• W4309631799 title "Chlorine-mediated synthesis of self-exfoliated and wavy-structured graphitic carbon nitride nanosheets for enhanced photocatalytic hydrogen evolution" @default.
• W4309631799 cites W1122398951 @default.
• W4309631799 cites W1515715292 @default.
• W4309631799 cites W1966753247 @default.
• W4309631799 cites W1979112470 @default.
• W4309631799 cites W1985201827 @default.
• W4309631799 cites W1990232236 @default.
• W4309631799 cites W2019851851 @default.
• W4309631799 cites W2042492216 @default.
• W4309631799 cites W2045182411 @default.
• W4309631799 cites W2051516460 @default.
• W4309631799 cites W2063836548 @default.
• W4309631799 cites W2078107904 @default.
• W4309631799 cites W2082579704 @default.
• W4309631799 cites W2085121573 @default.
• W4309631799 cites W2106595669 @default.
• W4309631799 cites W2115723858 @default.
• W4309631799 cites W2122198713 @default.
• W4309631799 cites W2132452349 @default.
• W4309631799 cites W2136661114 @default.
• W4309631799 cites W2146349866 @default.
• W4309631799 cites W2150399639 @default.
• W4309631799 cites W2161736606 @default.
• W4309631799 cites W2239593222 @default.
• W4309631799 cites W2292546454 @default.
• W4309631799 cites W2300593429 @default.
• W4309631799 cites W2323576468 @default.
• W4309631799 cites W2344538577 @default.
• W4309631799 cites W2399440163 @default.
• W4309631799 cites W2400670061 @default.
• W4309631799 cites W2401906193 @default.
• W4309631799 cites W2411369509 @default.
• W4309631799 cites W2442970291 @default.
• W4309631799 cites W2485549118 @default.
• W4309631799 cites W2497733926 @default.
• W4309631799 cites W2507619086 @default.
• W4309631799 cites W2517141693 @default.
• W4309631799 cites W2528439212 @default.
• W4309631799 cites W2617038631 @default.
• W4309631799 cites W2622155665 @default.
• W4309631799 cites W2794038766 @default.
• W4309631799 cites W2800003503 @default.
• W4309631799 cites W2893632787 @default.
• W4309631799 cites W2914251116 @default.
• W4309631799 cites W2921910176 @default.
• W4309631799 cites W3010304092 @default.
• W4309631799 cites W3083986413 @default.
• W4309631799 cites W3096342446 @default.
• W4309631799 cites W3108924328 @default.
• W4309631799 cites W3118497682 @default.
• W4309631799 cites W3137295689 @default.
• W4309631799 cites W3200155850 @default.
• W4309631799 doi "https://doi.org/10.1016/j.ijhydene.2022.10.235" @default.
• W4309631799 hasPublicationYear "2023" @default.
• W4309631799 type Work @default.
• W4309631799 citedByCount "1" @default.
• W4309631799 crossrefType "journal-article" @default.
• W4309631799 hasAuthorship W4309631799A5003642180 @default.
• W4309631799 hasAuthorship W4309631799A5012985474 @default.
• W4309631799 hasAuthorship W4309631799A5061575283 @default.
• W4309631799 hasAuthorship W4309631799A5073188500 @default.
• W4309631799 hasAuthorship W4309631799A5076596665 @default.
• W4309631799 hasAuthorship W4309631799A5083125123 @default.
• W4309631799 hasConcept C104779481 @default.
• W4309631799 hasConcept C127413603 @default.
• W4309631799 hasConcept C140205800 @default.
• W4309631799 hasConcept C159985019 @default.
• W4309631799 hasConcept C161790260 @default.
• W4309631799 hasConcept C171250308 @default.
• W4309631799 hasConcept C178790620 @default.
• W4309631799 hasConcept C179104552 @default.
• W4309631799 hasConcept C185592680 @default.
• W4309631799 hasConcept C191897082 @default.
• W4309631799 hasConcept C192562407 @default.
• W4309631799 hasConcept C194760766 @default.
• W4309631799 hasConcept C202189072 @default.
• W4309631799 hasConcept C2777492770 @default.
• W4309631799 hasConcept C2778835725 @default.
• W4309631799 hasConcept C2779227376 @default.
• W4309631799 hasConcept C42360764 @default.
• W4309631799 hasConcept C505241676 @default.
• W4309631799 hasConcept C512968161 @default.
• W4309631799 hasConcept C65165184 @default.
• W4309631799 hasConceptScore W4309631799C104779481 @default.
• W4309631799 hasConceptScore W4309631799C127413603 @default.
• W4309631799 hasConceptScore W4309631799C140205800 @default.
• W4309631799 hasConceptScore W4309631799C159985019 @default.
• W4309631799 hasConceptScore W4309631799C161790260 @default.

• next