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- W4309715462 abstract "Abstract Here, we report diversely fused oxa‐cages starting from various alkyl‐substituted cyclic‐ether derivatives derived via intramolecular cyclocetherification of endo ‐alcohol containing endo ‐norbornene derivatives. All these higher oxa‐cage systems are assembled in good to excellent yield by employing ring‐closing metathesis (RCM) or ring‐opening metathesis (ROM) as a key step. Ru‐based Grubbs catalysts (G‐I, G‐II) are effective to assemble these target molecules. In addition, a highly strained bicyclo[2.2.1]hepatane system fused oxa‐cages are easily prepared by hydrogenation sequence. Also, several highly fused saturated oxa‐cage derivatives are reported. A total of 22 examples are reported and all of these compounds are well‐characterized by NMR and HRMS data. The target compounds reported here may find significant applications in various fields of chemistry." @default.
- W4309715462 created "2022-11-29" @default.
- W4309715462 creator A5011215931 @default.
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- W4309715462 date "2022-12-07" @default.
- W4309715462 modified "2023-10-16" @default.
- W4309715462 title "Design and Synthesis of Highly Decorated Oxa‐Cage Systems via Olefin Metathesis" @default.
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- W4309715462 doi "https://doi.org/10.1002/ajoc.202200624" @default.
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