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- W4309730112 abstract "The Ni−Al bimetallic catalysis of intramolecular enantioselective and regioselective C−H cyclization of 4-oxoquinazolines with tethered alkenes has been successfully developed. Some new secondary phosphine oxides (SPOs) with large steric hindrance (SPO6-11) were designed and successfully synthesized from readily available chiral amines or amino acids. The developed chiral SPOs as ligands or preligands demonstrate much higher efficiency in the asymmetric catalytic reactions than the reported traditional ones. A new class of chiral tricyclic pyrroloquinazolinones were obtained in up to 95% yield and 99% ee." @default.
- W4309730112 created "2022-11-29" @default.
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- W4309730112 date "2023-06-01" @default.
- W4309730112 modified "2023-10-18" @default.
- W4309730112 title "Development of sterically hindered SPOs and enantioselective Ni−Al bimetallic catalyzed C−H cyclization of 4-oxoquinazolines with tethered alkenes" @default.
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- W4309730112 doi "https://doi.org/10.1016/j.cclet.2022.108017" @default.
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