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• W4309771268 endingPage "137353" @default.
• W4309771268 startingPage "137353" @default.
• W4309771268 abstract "A highly efficient heterogeneous electro-Fenton (Hetero-EF) catalyst with core-shell structure was successfully prepared by calcination of Mn-doped Mil-53 (Fe) precursor at high temperature. FeMn@C-800/2 prepared at pyrolysis temperature of 800 °C and Fe:Mn molar doping ratio of 2:1 showed the best catalytic performance for the degradation of carbamazepine (CBZ). The characterization, properties and stability of FeMn@C-800/2 were systematically investigated, obtaining the apparent first-order reaction rate of Hetero-EF was 8.9 and 17.8 times higher than that on Fe@C-800 and Mn@C-800 at the optimized conditions of current density 10 mA cm-2, catalyst dosage of 50 mg L-1 and initial pH 4.0, respectively. The incorporation of Mn promoted the generation of more Fe0 and Fe3C during the pyrolysis process, and enhanced the internal micro-electrolysis between Fe0 and carbon shell. At the same time, the presence of Mn0 also promoted the regeneration of Fe2+, and improved the activity of iron-carbon heterogeneous catalysis in the EF process, so as to degrade organic pollutants more effectively. This work would help to gain insight into the design of MOFs derived Fe-Mn bimetal catalyst and its mechanism for enhanced heterogeneous electro-Fenton." @default.
• W4309771268 created "2022-11-29" @default.
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• W4309771268 date "2023-01-01" @default.
• W4309771268 modified "2023-10-18" @default.
• W4309771268 title "Degradation of carbamazepine over MOFs derived FeMn@C bimetallic heterogeneous electro-Fenton catalyst" @default.
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• W4309771268 doi "https://doi.org/10.1016/j.chemosphere.2022.137353" @default.
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• W4309771268 hasPublicationYear "2023" @default.
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