FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4309773558> ?p ?o ?g. }

• W4309773558 endingPage "121202" @default.
• W4309773558 startingPage "121202" @default.
• W4309773558 abstract "In the past two decades, significant advancements have been made toward thin film fabrication of metal-organic frameworks (MOFs) on porous solid substrates for gas separation and catalysis applications. To enhance the physical and chemical stability of the films, various top-down and bottom-up approaches have been implemented. While both approaches have some advantages, they are mostly limited due to a lack of adhesion with the substrate, cracking of the films, and non-uniform coverages. Therefore, there is a need for improvement in the coating processes for the fabrication of robust, uniform, and scalable films. Here, we develop a novel percolation-assisted coating (PAC) process that combines top-down and bottom-up approaches in a continuous-flow microfluidic device to deposit HKUST-1 on a porous substrate, yielding controlled film thicknesses and mass loading. The PAC process is optimized using a Multiphysics modeling approach to design the microfluidic reactor, which can be readily scaled up and deployed to fabricate MOF films on various porous substrates. The desired thickness in the range of 10–200 μm of the MOF film can be achieved by controlling the residence time and temperature of the reaction mixture. The synthesized film is characterized for physical adhesion using sonication, film coverage using scanning electron microscopy, and porosity using a porosimeter. The performance of synthesized films is benchmarked for the effective separation of 50 vol% CH4–H2 gas mixture with the separation factor of 4. The microfluidic device is also applicable to synthesize films of various MOFs like MOF-5, MOF-505 (also reported here), UIO-66, etc., over a wide range of porous substrates. Lastly, we propose a multi-chamber design of the microfluidic device for high-throughput screening of thin-film growth using the PAC process." @default.
• W4309773558 created "2022-11-29" @default.
• W4309773558 creator A5001408049 @default.
• W4309773558 creator A5003372467 @default.
• W4309773558 creator A5024092825 @default.
• W4309773558 creator A5026993312 @default.
• W4309773558 creator A5049586249 @default.
• W4309773558 creator A5067490925 @default.
• W4309773558 creator A5090749959 @default.
• W4309773558 date "2023-02-01" @default.
• W4309773558 modified "2023-10-16" @default.
• W4309773558 title "Percolation-assisted coating of metal-organic frameworks on porous substrates" @default.
• W4309773558 cites W1974966064 @default.
• W4309773558 cites W1977442378 @default.
• W4309773558 cites W1977952172 @default.
• W4309773558 cites W2005588386 @default.
• W4309773558 cites W2069202835 @default.
• W4309773558 cites W2070043064 @default.
• W4309773558 cites W2081350764 @default.
• W4309773558 cites W2086855816 @default.
• W4309773558 cites W2101085407 @default.
• W4309773558 cites W2141939342 @default.
• W4309773558 cites W2168570857 @default.
• W4309773558 cites W2274399321 @default.
• W4309773558 cites W2329905093 @default.
• W4309773558 cites W2333883247 @default.
• W4309773558 cites W2472172567 @default.
• W4309773558 cites W2524029741 @default.
• W4309773558 cites W2554872674 @default.
• W4309773558 cites W2618702506 @default.
• W4309773558 cites W2733068487 @default.
• W4309773558 cites W2740668191 @default.
• W4309773558 cites W2772026629 @default.
• W4309773558 cites W2790292783 @default.
• W4309773558 cites W2791826355 @default.
• W4309773558 cites W2809781885 @default.
• W4309773558 cites W2883659932 @default.
• W4309773558 cites W2937062987 @default.
• W4309773558 cites W2939211090 @default.
• W4309773558 cites W2950543069 @default.
• W4309773558 cites W2971901360 @default.
• W4309773558 cites W2979569884 @default.
• W4309773558 cites W3037022972 @default.
• W4309773558 cites W3039136197 @default.
• W4309773558 cites W3086839938 @default.
• W4309773558 cites W3087890066 @default.
• W4309773558 cites W3119349227 @default.
• W4309773558 cites W3130272397 @default.
• W4309773558 cites W3134004591 @default.
• W4309773558 cites W3134975221 @default.
• W4309773558 cites W3163962155 @default.
• W4309773558 cites W3175266129 @default.
• W4309773558 cites W3203402166 @default.
• W4309773558 cites W4205780246 @default.
• W4309773558 cites W4206597312 @default.
• W4309773558 cites W4210935750 @default.
• W4309773558 cites W4211120562 @default.
• W4309773558 cites W4212784763 @default.
• W4309773558 cites W4214909249 @default.
• W4309773558 cites W4230501812 @default.
• W4309773558 doi "https://doi.org/10.1016/j.memsci.2022.121202" @default.
• W4309773558 hasPublicationYear "2023" @default.
• W4309773558 type Work @default.
• W4309773558 citedByCount "3" @default.
• W4309773558 countsByYear W43097735582023 @default.
• W4309773558 crossrefType "journal-article" @default.
• W4309773558 hasAuthorship W4309773558A5001408049 @default.
• W4309773558 hasAuthorship W4309773558A5003372467 @default.
• W4309773558 hasAuthorship W4309773558A5024092825 @default.
• W4309773558 hasAuthorship W4309773558A5026993312 @default.
• W4309773558 hasAuthorship W4309773558A5049586249 @default.
• W4309773558 hasAuthorship W4309773558A5067490925 @default.
• W4309773558 hasAuthorship W4309773558A5090749959 @default.
• W4309773558 hasConcept C105569014 @default.
• W4309773558 hasConcept C111368507 @default.
• W4309773558 hasConcept C114873805 @default.
• W4309773558 hasConcept C127313418 @default.
• W4309773558 hasConcept C127413603 @default.
• W4309773558 hasConcept C136525101 @default.
• W4309773558 hasConcept C142724271 @default.
• W4309773558 hasConcept C159985019 @default.
• W4309773558 hasConcept C169760540 @default.
• W4309773558 hasConcept C171250308 @default.
• W4309773558 hasConcept C19067145 @default.
• W4309773558 hasConcept C192562407 @default.
• W4309773558 hasConcept C204787440 @default.
• W4309773558 hasConcept C2777289219 @default.
• W4309773558 hasConcept C2780457167 @default.
• W4309773558 hasConcept C2781448156 @default.
• W4309773558 hasConcept C42360764 @default.
• W4309773558 hasConcept C6648577 @default.
• W4309773558 hasConcept C71924100 @default.
• W4309773558 hasConcept C8673954 @default.
• W4309773558 hasConcept C86803240 @default.
• W4309773558 hasConceptScore W4309773558C105569014 @default.
• W4309773558 hasConceptScore W4309773558C111368507 @default.
• W4309773558 hasConceptScore W4309773558C114873805 @default.
• W4309773558 hasConceptScore W4309773558C127313418 @default.

• next