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- W4309774285 abstract "Preparing highly efficient electrocatalysts via structural or electronic manipulation always holds great interest in water electrolyzers. Here, we introduce the non-precious Na atoms to NiFe-LDH and investigate the effect of electronic configuration changes on electrocatalytic water oxidation. The electrochemical tests reveal that the NiFe-LDH monolayer decorated with Na atoms (Na/NiFe-LDH) possesses superior oxygen evolution reaction (OER) performance, achieving an overpotential of 279 mV at the current density of 100 mA cm−2. The experimental characterizations highlight the effect of the Na-O3 motif on improving the intrinsic OER activity and facilitating surface charge transfer kinetics. Further theoretical calculations confirm that the formation of the Na-O3 motif reduces the strength of the Fe-O bond in the NiFe-LDH skeleton and induces the spin-state inversion for Fe 3d orbitals, which accounts for the enhanced OER performance. This work demonstrates an effective method to enhance the OER activity of NiFe-LDH through spin-state regulation." @default.
- W4309774285 created "2022-11-29" @default.
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- W4309774285 date "2023-02-01" @default.
- W4309774285 modified "2023-09-27" @default.
- W4309774285 title "Spin-state inversion in non-precious Na single atoms decorated NiFe-LDH monolayer for efficient electrocatalytic water oxidation" @default.
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- W4309774285 doi "https://doi.org/10.1016/j.apsusc.2022.155751" @default.
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