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- W4309780248 abstract "• Coupled energy-saving H 2 production and electro-synthesis of energetic compound. • Ru single atoms loaded on MoS 2 nanosheets on carbon cloth substrate for HER. • DFT attribute the performance to charge redistribution and synergistic interaction. The electrochemical water splitting process is comprised of hydrogen evolution reaction (HER) and oxygen evolution reaction (OER), where the OER is usually the bottleneck of the whole reaction, causing the high overpotential, while the oxidation product (O 2 ) is of less economic value. In this article, we report a new coupling system based on the green electro-oxidation synthesis of energetic compounds and simultaneous H 2 production on the molybdenum disulfide/ruthenium-based single-atom catalyst (Ru SAs MoS 2 /CC). The charge redistribution and synergistic interaction between MoS 2 and Ru SAs for alkaline HER were systemically investigated by experimental and density functional theory (DFT) calculation. More importantly, the integration of overall water splitting (OWS) and anodic N-N oxidative coupling of 5-amino-1 H -tetrazole (5-AT) shows an ultralow cell voltage of 1.36 V at 10 mA cm –2 for the H 2 production and simultaneously realize green-synthesis of dipotassium 5,5′-azotetrazole (K 2 AZT), which is traditionally synthesized under harsh condition requiring high temperature and excessive oxidant. This work highlights a unique strategy for energy-saving H 2 production and eco-friendly electrosynthesis of energetic compounds." @default.
- W4309780248 created "2022-11-29" @default.
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- W4309780248 date "2023-02-01" @default.
- W4309780248 modified "2023-10-04" @default.
- W4309780248 title "Green N-N oxidative coupling synthesis of energetic compounds and energy-saving hydrogen evolution reaction" @default.
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- W4309780248 doi "https://doi.org/10.1016/j.apsusc.2022.155659" @default.
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